Recycling and Reinforcement of Retired EV Battery Materials in Polymer Composites for Sustainable Engineering Applications

Notice

This is an unedited manuscript accepted for publication and provided as an Article in Press for early access at the author’s request. The article will undergo copyediting, typesetting, and galley proof review before final publication. Please be aware that errors may be identified during production that could affect the content. All legal disclaimers of the journal apply.

Year : 2026 | Volume : 14 | 03 | Page :
    By

    Rajkumar K. Chougale,

  • Pralhad B. Patole,

  • Amit A. Desai,

  • Gayatri S. Ghorpade,

  • Balaji T. Mohite,

  • Jayant C. Thorat,

  1. Assistant Professor, Department of Electrical Engineering, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India
  2. Associate Professor, Department of Mechanical Engineering, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India
  3. Assistant Professor, Department of Mechanical Engineering, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India
  4. Assistant Professor, Department of Environmental science, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India
  5. Assistant Professor, Department of Mathematics, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India
  6. Assistant Professor, Department of Chemistry, Bharati Vidyapeeth’s College of Engineering, Kolhapur, Maharashtra, India

Abstract

The rapid proliferation of electric vehicles (EVs) has led to a substantial increase in lithium-ion battery waste, necessitating sustainable strategies for material recovery and reuse. This review explores the valorization of retired Electrical Vehicle batteries within polymer and composite systems, highlighting second-life applications as a promising pathway toward circular material utilization. Batteries retaining 70–80% of their original capacity remain suitable for extended use; however, beyond conventional energy storage, their constituent materials—including electrode powders, current collectors, and separators—can be effectively incorporated into polymer matrix composites for both functional and structural applications. This study critically examines battery degradation mechanisms, material recovery processes, and the transformation of recovered components into composite fillers and reinforcements. Particular emphasis is placed on polymer–battery material interactions, processing techniques such as melt blending and solution casting, and the resulting mechanical, electrical, and thermal properties of the developed composites. Techno-economic analysis demonstrates the feasibility of cost-effective material substitution, while life cycle assessment highlights significant environmental benefits, including reduced carbon footprint and conservation of critical raw materials. Emerging strategies, including hybrid composite systems, conductive polymers, and multifunctional materials, are discussed alongside key challenges such as material heterogeneity, interfacial compatibility, and large-scale scalability.

Finally, This strategy not only mitigates the environmental burden associated with battery waste but also promotes resource circularity by converting end-of-life materials into value-added functional components. the integration of retired EV battery materials into polymer composites represents a novel and high-impact approach, advancing sustainable materials engineering and efficient energy resource management for future technologies.

Keywords: Recycling, Reinforcement, Polymer Composites, Sustainable Engineering

How to cite this article:
Rajkumar K. Chougale, Pralhad B. Patole, Amit A. Desai, Gayatri S. Ghorpade, Balaji T. Mohite, Jayant C. Thorat. Recycling and Reinforcement of Retired EV Battery Materials in Polymer Composites for Sustainable Engineering Applications. Journal of Polymer & Composites. 2026; 14(03):-.
How to cite this URL:
Rajkumar K. Chougale, Pralhad B. Patole, Amit A. Desai, Gayatri S. Ghorpade, Balaji T. Mohite, Jayant C. Thorat. Recycling and Reinforcement of Retired EV Battery Materials in Polymer Composites for Sustainable Engineering Applications. Journal of Polymer & Composites. 2026; 14(03):-. Available from: https://journals.stmjournals.com/jopc/article=2026/view=245065


References

  1. Udendhran, R., Mohan, T. R., R, B., et al., (2025b). Transitioning to sustainable E-vehicle systems – Global perspectives on the challenges, policies, and opportunities. Journal of Hazardous Materials Advances, 17, 100619. https://doi.org/10.1016/j.hazadv.2025.100619
  2. International Energy Agency. Global EV Outlook 2024: Outlook for Battery and Energy Demand [Internet]. Paris: IEA; 2024. Available from: https:// iea.org/reports/global-ev-outlook-2024
  3. Global battery demand to quadruple by 2030 and OEMs must hone in on their battery strategies. (n.d.). Bain. https://www.bain.com/about/media-center/press-releases/2024/global-battery-demand-to-quadruple-by-2030-and-oems-must-hone-in-on-their-battery-strategies/
  4. Zhu J, Mathews I, Ren D, Li W, et al. (2021). End-of-life or second- life options for retired electric vehicle batteries. Cell Rep Phys Sci. 2021;2(11):
  5. Neubauer JS, Wood E, Pesaran A. (2015). A second life for electric vehicle batteries: answering questions on battery degradation and SAE Int J Mater Manuf. 2015;8(2):544-53.
  6. Iqbal H, Sarwar S, Kirli D, Shek JKH, Kiprakis AE. A survey of second-life batteries based on techno-economic perspective and applications-based analysis. Carbon Neutrality. 2023;2:49.
  7. Preger Y, Barkholtz HM, Fresquez A, Campbell DL, Jansz K, Ferreira SR, et al. Degradation of commercial lithium-ion cells as a function of chemistry and cycling conditions. J Electrochem Soc. 2020;167(12):120532.
  8. Koech, A. K., Mwandila, G., & Mulolani, F. (2024). A review of improvements on electric vehicle battery. Heliyon, 10(15), e34806. https://doi.org/10.1016/j.heliyon.2024.e34806
  9. Chowdhury, C. R., Biswas, A., Kibria, M. G., & Mourshed, M. (2026). Battery waste management: Tackling environmental, health, and resource challenges from growing waste. Chemical Engineering Journal Advances, 25, 101033. https://doi.org/10.1016/j.ceja.2026.101033
  10. Elmahallawy M, Elfouly T, Alouani A, et al., (2022). A comprehensive review of lithium-ion batteries modeling, and state of health and remaining useful lifetime prediction. IEEE Access. 10:113259-113295.
  11. Preger Y, Barkholtz HM, Fresquez A, et al. (2020). Degradation of commercial lithium-ion cells as a function of chemistry and cycling conditions. J Electrochem Soc. 167(12):120532.
  12. John J, Kudva G, Jayalakshmi NS. (2024). Secondary life of electric vehicle batteries: degradation, state of health estimation using incremental capacity analysis, applications and challenges. IEEE Access. 12:54826-54852.
  13. Jameel SM, Altmemi JM, Oglah AA, et al., (2024). Predicting batteries second-life state-of-health with first-life data and on-board voltage measurements using support vector regression. J Energy Storage. 86:111103.
  14. Wei J, Dong G, Chen Z. Remaining useful life prediction and state of health diagnosis for lithium-ion batteries using particle
  15. Palanisamy, S., Kalimuthu, M., Azeez, A., et al., (2022). Wear properties and Post-Moisture absorption mechanical behavior of KENAF/Banana-Fiber-Reinforced epoxy composites. Fibers, 10(4), 32. https://doi.org/10.3390/fib10040032
  16. Aruchamy, K., Karuppusamy, M., Krishnakumar, S., et al., (2024). Enhancement of mechanical properties of hybrid polymer composites using palmyra palm and coconut sheath fibers: The role of tamarind shell powder. BioResources, 20(1), 698–724. https://doi.org/10.15376/biores.20.1.698-724
  17. Ayrilmis, N., Kanat, G., Avsar, E. Y., et al., (2024). Utilizing waste manhole covers and fibreboard as reinforcing fillers for thermoplastic composites. Journal of Reinforced Plastics and Composites, 44(17–18), 1108–1118. https://doi.org/10.1177/07316844241238507
  18. Ramasubbu, R., Kayambu, A., Palanisamy, S., & Ayrilmis, N. (2024). Mechanical properties of epoxy composites reinforced with Areca catechu fibers containing silicon carbide. BioResources, 19(2), 2353–2370. https://doi.org/10.15376/biores.19.2.2353-2370
  19. Palanisamy, S., Murugesan, T. M., Palaniappan, M., Santulli, C., & Ayrilmis, N. (2024). Fostering sustainability: The environmental advantages of natural fiber composite materials – a mini review. Environmental Research and Technology, 7(2), 256–269. https://doi.org/10.35208/ert.1397380
  20. Yu, K., Yan, P., Liu, Y., Chen, Z., & Kong, X. T. (2025). Battery degradation mitigation-oriented strategy for optimizing e-hailing electric vehicle operations. Transportation Research Part E Logistics and Transportation Review, 196, 104006. https://doi.org/10.1016/j.tre.2025.104006
  21. Jameel SM, Altmemi JM, Oglah AA, et al., (2024). Predicting batteries second-life state-of-health with first-life data and on-board voltage measurements using support vector regression. J Energy Storage. 86:111103.
  22. Wei J, Dong G, Chen Z. (2017). Remaining useful life prediction and state of health diagnosis for lithium-ion batteries using particle filter and support vector regression. IEEE Trans Ind Electron. 65(7):5634-5643.
  23. Casals LC, García BA, Aguesse F, et al., (2017). Second life of electric vehicle batteries: relation between materials degradation and environmental impact. Int J Life Cycle Assess. 22:82-93.
  24. Lin CP, Cabrera J, Yang F, et al., (2020). Battery state of health modeling and remaining useful life prediction through time series model. Appl Energy. 275:115398.
  25. Börner MF, Frieges MH, Späth B, et al., (2022). Challenges of second-life concepts for retired electric vehicle batteries. Cell Rep Phys Sci. 2022;3(8):101039.
  26. Reschiglian T, Sevdari K, et al. (2024). Repurposing Second Life EV Battery for Stationary Energy Storage Applications. In: 2024 IEEE PES Innovative Smart Grid Technologies Conference; 2024.
  27. Yu M, Bai B, Xiong S, Liao X. (2021). Evaluating environmental impacts and economic performance of remanufacturing electric vehicle lithium-ion batteries. J Clean Prod. 315:128099.
  28. Wu W, Lin B, Xie C, Elliott RJR, Radcliffe J. (2021). Does energy storage provide a profitable second life for electric vehicle batteries? Energy Econ. 97:105182.
  29. Dini, P., Colicelli, A., & Saponara, S. (2024). Review on Modeling and SOC/SOH Estimation of batteries for Automotive Applications. Batteries, 10(1), 34. https://doi.org/10.3390/batteries10010034
  30. Jiang, Y. (2026). A review of secondary utilization of retired power battery. Applied and Computational Engineering, 221(1), 193–205. https://doi.org/10.54254/2755-2721/2026.mh31663
  31. Horesh N, Quinn C, Wang H, et al. (2021). Driving to the future of energy storage: techno-economic analysis of a novel method to recondition second life electric vehicle batteries. Appl Energy. 299:117300.
  32. Patel AN, Lander L, Ahuja J, et al., (2024). Lithium-ion battery second life: pathways, challenges and outlook. Front Chem. 8;12:1358417. doi: 10.3389/fchem.2024.1358417.
  33. Attia PM, Moch E, Herring PK. Challenges and opportunities for high-quality battery production at scale. Nat Commun. 2025 Jan 12;16(1):611. doi: 10.1038/s41467-025-55861-7
  34. S, S. B., Hampannavar, S., B, D., & Bairwa, B. (2022). Applications of Battery Management System (BMS) in Sustainable Transportation: A Comprehensive Approach from Battery Modeling to Battery Integration to the Power Grid. World Electric Vehicle Journal, 13(5), 80. https://doi.org/10.3390/wevj13050080
  35. Akhtar, M., Shahzadi, S., Arshad, M., Akhtar, T., & Janjua, M. R. S. A. (2025). Metal oxide-polymer hybrid composites: a comprehensive review on synthesis and multifunctional applications. RSC Advances, 15(23), 18173–18208. https://doi.org/10.1039/d5ra01821h
  36. Natarajan, S., Lakshmi, D. S., Bajaj, H. C., & Srivastava, D. N. (2015). Recovery and utilization of graphite and polymer materials from spent lithium-ion batteries for synthesizing polymer–graphite nanocomposite thin films. Journal of Environmental Chemical Engineering, 3(4), 2538–2545. https://doi.org/10.1016/j.jece.2015.09.011
  37. Abdelbaky M, Peeters JR, Dewulf W. (2021). On the influence of second use, future battery technologies, and battery lifetime on the maximum recycled content of future electric vehicle batteries in Europe. Waste Manage. 130:24-35.
  38. Yi, C., Zhou, L., Wu, X., et al., (2021). Technology for recycling and regenerating graphite from spent lithium-ion batteries. Chinese Journal of Chemical Engineering, 39, 37–50. https://doi.org/10.1016/j.cjche.2021.09.014
  39. Mathiyalagan, R., & Kandasamy, J. (2026). EV battery recycling economics and rare earth element recovery for sustainable resource management. Discover Sustainability, 7(1). https://doi.org/10.1007/s43621-026-02662-7
  40. Kotak, Y., Fernández, C. M., Casals, L. C., et al., (2021). End of Electric Vehicle Batteries: Reuse vs. Recycle. Energies, 14(8), 2217. https://doi.org/10.3390/en14082217
  41. Abdelbaky M, Peeters JR, Dewulf W. (2021). On the influence of second use, future battery technologies, and battery lifetime on the maximum recycled content of future electric vehicle batteries in Europe. Waste Manage. 130:24-35.
  42. Lehmusto, M., & Santasalo-Aarnio, A. (2025). Impact of first-life usage on second-life performance of lithium-ion batteries. Next Energy, 9, 100385. https://doi.org/10.1016/j.nxener.2025.100385
  43. Kang, Z., Huang, Z., Peng, Q., et al.,  (2023). Recycling technologies, policies, prospects, and challenges for spent batteries. iScience, 26(11), 108072. https://doi.org/10.1016/j.isci.2023.108072
  44. Zhao, H., Zuo, H., Wang, J., & Jiao, S. (2024). Practical application of graphite in lithium-ion batteries: Modification, composite, and sustainable recycling. Journal of Energy Storage, 98, 113125. https://doi.org/10.1016/j.est.2024.113125
  45. Custom Market Insights. Second-life EV Batteries Market Size, Share 2030 [Internet]. 2024. Available from: https://www.custommarketinsights.com/ report/second-life-ev-batteries-market/
  46. Goudar, J. A., SN, T., Chapi, S., et al., (2025). Ferrite-polymer composites: A novel approach to high-performance energy storage materials. Next Energy, 8, 100367. https://doi.org/10.1016/j.nxener.2025.100367
  47. Srinivasan, S., Shanthakumar, S., & Ashok, B. (2024). Sustainable lithium-ion battery recycling: A review on technologies, regulatory approaches and future trends. Energy Reports, 13, 789–812. https://doi.org/10.1016/j.egyr.2024.12.043
  48. Ngoy, K. R., Lukong, V. T., Yoro, K. O., et al., (2025). Lithium-ion batteries and the future of sustainable energy: A comprehensive review. Renewable and Sustainable Energy Reviews, 223, 115971. https://doi.org/10.1016/j.rser.2025.115971
  49. Laad M, Sur A, Kale G, et al., (2025). Synthesis and characterization of carbon based polymer composites reinforced with MWCNTs and graphite in PVDF matrix. Sci Rep. 15(1):28928. doi: 10.1038/s41598-025-13421-5
  50. Chen, J., Mohammed, K. J., Ali, E., & Marzouki, R. (2025). Carbon additives to improve polymer performance in energy applications using machine learning. Case Studies in Construction Materials, 23, e05099. https://doi.org/10.1016/j.cscm.2025.e05099
  51. Neumann J, Petranikova M, Meeus M, et al., (2022). Recycling of lithium-ion batteries—current state of the art, circular economy, and next generation recycling. Adv Energy Mater. 12(17):2102917.
  52. Edge, J. S., O’Kane, S., Prosser, R., et al., (2021b). Lithium ion battery degradation: what you need to know. Physical Chemistry Chemical Physics, 23(14), 8200–8221. https://doi.org/10.1039/d1cp00359c
  53. Braco E, San Martín I, Berrueta A, et al., (2021). Experimental assessment of first-and second-life electric vehicle batteries: performance, capacity dispersion, and aging. IEEE Trans Ind Appl. 57(4): 4285-4294.
  54. Kelly, N., et al., (2026). Hydrometallurgical recovery of high-purity copper from waste printed circuit boards: an experimental study and life cycle assessment. Environmental Science Advances, 5(3), 772–790. https://doi.org/10.1039/d5va00348b
  55. Wang Y, Tang B, Shen M, Wu Y, et al., (2022). Environmental impact assessment of second life and recycling for LiFePO4 power batteries in China. J Environ Manage. 315:115245.
  56. Hellmuth JF, DiFilippo NM, Jouaneh MK. (2021). Assessment of the automation potential of electric vehicle battery disassembly. J Manuf Syst. 2021;61:24-34.
  57. Turan F, Boynuegri AR, Durmaz T. Comprehensive technical and economic evaluations of using second-life batteries as energy storage in off-grid applications: a customized cost analysis. J Energy Storage. 2025;106:113928.
  58. Custom Market Insights. Second-life EV Batteries Market Size, Share 2030 [Internet]. 2024. Available from: https://www.custommarketinsights.com/ report/second-life-ev-batteries-market/
  59. Kannapiran, E., Joshi, K., Chougale, R. K., et al., (2022). Smart Electric vehicle charging Station for Residential Complex. 2022 International Conference on Innovative Computing, Intelligent Communication and Smart Electrical Systems (ICSES). https://doi.org/10.1109/icses55317.2022.9914182
  60. Pagliaro M, Meneguzzo F. (2019). Lithium battery reusing and recycling: a circular economy insight. Heliyon. 5(6):e01866.
  61. Harper GDJ, Kendrick E, Anderson PA, Harper GDJ. (2023). Roadmap for a sustainable circular economy in lithium-ion and future battery technologies. J Phys Energy. 5(2):022001.
  62. Hildebrand S, Eddarir A, Lebedeva N. (2024). Overview of battery safety tests in standards for stationary battery energy storage systems [Internet]. Available from: https://www.researchgate.net/
  63. Mylenbusch IS, Claffey K, Chu BN. (2023). Hazards of lithium-ion battery energy storage systems (BESS), mitigation strategies, minimum requirements, and best practices. Process Saf Prog. 42(2):180-195.
  64. Dawson L, Ahuja J, Lee R. (2021). Steering extended producer responsibility for electric vehicle batteries. Environ Law Rev. 23(2):89-106.
  65. Turner JM, Nugent LM. (2016). Charging up battery recycling policies: extended producer responsibility for single-use batteries in the European union, Canada, and the United States. J Ind Ecol. 20(5):1146-1158.
  66. Kostenko G, Zaporozhets A. (2024). World experience of legislative regulation for lithium-ion electric vehicle batteries considering their second-life application in power sector. Syst Res Energy. 14:836.
  67. Saez-de-Ibarra A, Martinez-Laserna E, Stroe DI, et al., (2024). Evaluation of the second-life potential of the first- generation Nissan Leaf battery packs. Energy Rep. 11:100031.
  68. Steckel T, Kendall A, Ambrose H. (2021). Applying levelized cost of storage methodology to utility-scale second-life lithium-ion battery energy storage systems. Appl Energy. 300:117314.

Ahead of Print Subscription Review Article
Volume 14
03
Received 24/04/2026
Accepted 12/05/2026
Published 22/05/2026
Publication Time 28 Days


Login


My IP

PlumX Metrics