Magnetic Metal–Polymer Composites with Ferromagnetic Particle Networks for EMI Shielding in Flexible Electronics

Year : 2026 | Volume : 14 | Issue : 01 | Page : 25 39
    By

    Kedri Janardhana,

  • P. Suresh Kumar,

  • Santhi M George,

  • B Karthik,

  • P.Duraipandy,

  • Kode Jaya Prakash,

  • Gadhamsetty Gurumahesh,

  • Sathish Rengarajan,

  • Sekar K,

  1. Assistant Professor (Selection Grade), Department of Electrical Engineering, Faculty of Engineering, Dayalbagh Educational Institute (Deemed to be University), Agra, Uttar Pradesh, India
  2. Associate Professor, Department of Mechanical Engineering, R. V. R & J. C. College of Engineering, Guntur, Andhra Pradesh, India
  3. Associate Professor, Department of Science and Humanities, R.M.K. Engineering College, Kavaraipettai, Tamil Nadu, India
  4. Associate Professor, Department of Electrical and Electronics Engineering, Sona College of Technology, Salem, Tamil Nadu, India
  5. Associate Professor, Department of Electrical and Electronics Engineering, J. B. Institute of Engineering and Technology, Hyderabad, Telangana, India
  6. Senior Assistant Professor, Department of Mechanical Engineering, VNR Vignana Jyothi Institute of Engineering & Technology, Hyderabad, Telangana, India
  7. Associate Professor, Department of Mechanical Engineering, Sri Venkateswara College of Engineering, Tirupati, Andhra Pradesh, India
  8. Professor, Department of Mechanical Engineering, St.Joseph’s College of Engineering, OMR, Chennai, Tamil Nadu, India
  9. Professor, Department of Electrical and Electronics Engineering, Adithya Institute of Technology, Coimbatore, Tamil Nadu, India

Abstract

The rapid expansion of flexible and wearable electronic systems has intensified the demand for lightweight, mechanically compliant materials capable of effective electromagnetic interference (EMI) shielding. In this study, magnetic metal–polymer composites with magnetically aligned ferromagnetic particle networks were developed and systematically investigated for EMI shielding in flexible electronics. Thermoplastic polyurethane (TPU) was employed as an elastomeric polymer matrix due to its excellent flexibility, dielectric characteristics, and compatibility with particulate fillers. Ferromagnetic Fe₃O₄ and Ni fillers were incorporated and aligned using a magnetic field-assisted assembly strategy to transform the polymer composite architecture from a randomly dispersed particulate system into a network-dominated functional composite. Magnetic, electrical, mechanical, and EMI shielding properties were evaluated to establish clear structure–property relationships. The aligned polymer composites exhibited enhanced saturation magnetization and reduced electrical percolation thresholds, confirming efficient network formation within the polymer matrix. EMI shielding effectiveness exceeded 40 dB in the X-band (8–12 GHz) at optimized filler loadings, corresponding to over 99.99% electromagnetic attenuation. Importantly, shielding was dominated by absorption rather than reflection, arising from synergistic magnetic losses, interfacial polarization, and polymer dielectric dissipation. Despite increased stiffness at higher filler contents, the polymer composites retained high elongation at break (>300%), demonstrating excellent flexibility and mechanical durability. Overall, the results highlight that polymer composite architecture, rather than filler content alone, governs EMI shielding performance. The combination of elastomeric TPU matrices and magnetically engineered ferromagnetic networks provides a scalable and mechanically robust pathway for next-generation flexible EMI shielding materials.

Keywords: EMI shielding, ferromagnetic networks, flexible electronics, metal–polymer composites, shielding properties

[This article belongs to Journal of Polymer & Composites ]

How to cite this article:
Kedri Janardhana, P. Suresh Kumar, Santhi M George, B Karthik, P.Duraipandy, Kode Jaya Prakash, Gadhamsetty Gurumahesh, Sathish Rengarajan, Sekar K. Magnetic Metal–Polymer Composites with Ferromagnetic Particle Networks for EMI Shielding in Flexible Electronics. Journal of Polymer & Composites. 2026; 14(01):25-39.
How to cite this URL:
Kedri Janardhana, P. Suresh Kumar, Santhi M George, B Karthik, P.Duraipandy, Kode Jaya Prakash, Gadhamsetty Gurumahesh, Sathish Rengarajan, Sekar K. Magnetic Metal–Polymer Composites with Ferromagnetic Particle Networks for EMI Shielding in Flexible Electronics. Journal of Polymer & Composites. 2026; 14(01):25-39. Available from: https://journals.stmjournals.com/jopc/article=2026/view=236218


References

  1. Seetha Rama Raju V, Kandukuri S, Singh AK, Satya Narayana Murthy V. Magnetic-polymer flexible composites for electromagnetic interference shielding applications. J Mater Sci Mater Electron. 2024;35(32):2067.
  2. Drozdov AD, deClaville Christiansen J. Electromagnetic properties and EMI shielding effectiveness of polymer composites reinforced with ferromagnetic particles at microwave frequencies. J Appl Phys. 2020;127(12):125103.
  3. Lu QW, Macosko CW. Comparing the compatibility of various functionalized polypropylenes with thermoplastic polyurethane. Polymer. 2004;45(6):1981–1991.
  4. Ahad NA. A recent blend of thermoplastic polyurethane. In: IOP Conf Ser Mater Sci Eng. 2020;957(1):012045.
  5. Xu T, Shen W, Lin X, Xie YM. Mechanical properties of additively manufactured thermoplastic polyurethane material affected by various processing parameters. Polymers. 2020;12(12):3010.
  6. Desai SM, Sonawane RY, More AP. Thermoplastic polyurethane for three-dimensional printing applications: a review. Polym Adv Technol. 2023;34(7):2061–2082.
  7. Kumar P, Narayan Maiti U, Sikdar A, Das TK, Kumar A, Sudarsan V. Recent advances in polymer and polymer composites for electromagnetic interference shielding: review and future prospects. Polym Rev. 2019;59(4):687–738.
  8. Yao Y, Jin S, Wang D, Wang J, Li D, Lv X, Shu Q. Flexible magnetoelectric coupling nanocomposite films with multilayer network structure for dual-band EMI shielding. Compos Sci Technol. 2022;222:109387.
  9. Nan Z, Wei W, Lin Z, Chang J, Hao Y. Flexible nanocomposite conductors for electromagnetic interference shielding. Nano Micro Lett. 2023;15(1):172.
  10. Sambhudevan S. Ferrite-based polymer nanocomposites as shielding materials: a review. Chem Pap. 2021;75(8):3697–3710.
  11. Wang L, Ma Z, Zhang Y, Chen L, Cao D, Gu J. Polymer-based EMI shielding composites with 3D conductive networks: a mini-review. SusMat. 2021;1(3):413–431.
  12. Yao Y, Jin S, Zou H, Li L, Ma X, Lv G, et al. Polymer-based lightweight materials for electromagnetic interference shielding: a review. J Mater Sci. 2021;56(11):6549–6580.
  13. Zhan Y, Santillo C, Meng Y, Lavorgna M. Recent advances and perspectives on silver-based polymer composites for electromagnetic interference shielding. J Mater Chem C. 2023;11(3):859–892.
  14. Charles AD. Advancing particle-based magneto-polymer composites: processing, structure, and performance optimisation for actuation, EMI suppression, and energy transduction [dissertation]. Sydney: University of New South Wales; 2023.
  15. Zhang Q, Wu Y, Bao X, Li S, Zhuang X, He Z, et al. High-performance, strain-stable electromagnetic shielding materials enabled by magnetic elastic fiber networks pinning liquid metal. Adv Sci. 2025;12(38):e10078.
  16. Zhu H, Yang Y, Duan H, Zhao G, Liu Y. Electromagnetic interference shielding polymer composites with magnetic and conductive FeCo/reduced graphene oxide 3D networks. J Mater Sci Mater Electron. 2019;30(3):2045–2056.
  17. Wanasinghe D, Aslani F, Ma G, Habibi D. Review of polymer composites with diverse nanofillers for electromagnetic interference shielding. Nanomaterials. 2020;10(3):541.
  18. Shukla V. Review of electromagnetic interference shielding materials fabricated by iron ingredients. Nanoscale Adv. 2019;1(5):1640–1671.
  19. Anand S, Pauline S. Electromagnetic interference shielding properties of BaCo₂Fe₁₆O₂₇ nanoplatelets and RGO reinforced PVDF polymer composite flexible films. Adv Mater Interfaces. 2021;8(3):2001810.
  20. Caramitu AR, Ciobanu RC, Ion I, Schreiner CM, Aradoaei M, Tsakiris V, et al. Flexible electromagnetic shielding nanocomposites based on silicon and NiFe₂O₄ powders. Polymers. 2023;15(11):2447.
  21. Kruželák J, Kvasničáková A, Hložeková K, Hudec I. Progress in polymers and polymer composites used as efficient materials for EMI shielding. Nanoscale Adv. 2021;3(1):123–172.
  22. Bheema RK, Gopu J, Bhaskaran K, Verma A, Chavali M, Etika KC. Recent progress in polymer composites for effective electromagnetic interference shielding: structures, processes, and sustainability approaches. Nanoscale Adv. 2024;6(23):5773–5802.
  23. Lyu L, Liu J, Liu H, Liu C, Lu Y, Sun K, et al. Electrically conductive polymer nanocomposites toward electromagnetic interference shielding: an overview. Eng Sci. 2018;2:26–42.
  24. Prajapati V, Yadav K, Abhyankar AC, Kandasubramanian B. PVDF-based electrospun composite material for electromagnetic interference shielding applications. Polym Plast Technol Mater. 2022;61(3):296–305.
  25. Zhan Y, Wang J, Zhang K, Li Y, Meng Y, Yan N, et al. Flexible EMI shielding Fe₃O₄@reduced graphene oxide/natural rubber composites with segregated networks. Chem Eng J. 2018;344:184–193.
  26. Wang H, Li S, Liu M, Li J, Zhou X. Shielding mechanisms and structural design of electromagnetic interference shielding composites: a review. Macromol Mater Eng. 2021;306(6):2100032.
  27. Wei H, Wang H, Li A, Cui D, Zhao Z, Chu L, et al. Multifunctional polymer nanocomposites for environmental remediation, EMI shielding, and sensing. ChemNanoMat. 2020;6(2):174–184.
  28. Zhang N, Zhao R, He D, Ma Y, Qiu J, Jin C, et al. Lightweight and flexible Ni–Co alloy nanoparticle-coated electrospun polymer nanofiber membranes for high-performance EMI shielding. J Alloys Compd. 2019;784:244–255.
  29. Sambyal P, Noh SJ, Hong JP, Kim WN, Iqbal A, Hwang SS, et al. FeSiAl/metal core–shell hybrid composites with high-performance EMI shielding. Compos Sci Technol. 2019;172:66–73.
  30. Arief I, Bhattacharjee Y, Prakash O, Sahu M, Suwas S, Bose S. Tunable CoNi microstructures in flexible multilayered polymer films for electromagnetic radiation shielding. Compos Part B Eng. 2019;177:107283.
  31. Jasna M, Pushkaran NK, Manoj M, Aanandan CK, Jayaraj MK. Lightweight and flexible PVA/PEDOT:PSS/MWCNT ternary composites for high-performance EMI shielding in the X-band. J Electron Mater. 2020;49(3):1856–1866.
  32. Chaudhary A, Kumar R, Teotia S, Dhawan SK, Dhakate SR, Kumari S. MCMBs/MWCNTs–Fe₃O₄ integrated flexible composite paper for electromagnetic interference shielding. J Mater Chem C. 2017;5(2):322–332.

Regular Issue Subscription Original Research
Volume 14
Issue 01
Received 20/12/2025
Accepted 07/01/2026
Published 17/01/2026
Publication Time 28 Days


Login


My IP

PlumX Metrics