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A Chandrashekhar,
K. Arun,
Om Prakash Sharma,
Rathinamala S,
Mallikarjunarao Dandu,
M. Premalatha,
P Joel Josephson,
G.Nixon Samuel Vijayakumar,
Rajendiran M,
- Associate Professor, Department of Mechanical Engineering, Faculty of Science and Technology, Icfai Foundation for Higher Education, Hyderabad, Telangana, India
- Associate Professor, Department of Mechanical Engineering, St. Joseph’s College of Engineering, Chennai, Tamil Nadu, India
- Professor, Faculty of Engineering and Technology, Jagan Nath University, Jaipur, Rajasthan, India
- Professor, Department of Electrical and Electronics Engineering, Kalaignarkarunanidhi Institute of Technology, Kannampalayam, Tamil Nadu, India
- Assistant Professor, Department of Mechanical Engineering, Lakireddy Bali Reddy College of engineering, Mylavaram, Andhra Pradesh, India
- Associate Professor, Department of Mathematics, Vel Tech Rangarajan Dr. Sagunthala R&D Institute of Science and Technology, Chennai, Tamil Nadu, India
- Associate Professor, Department of Electronics and Communication Engineering, Malla Reddy (MR) Deemed to be University, Hyderabad, Telangana, India
- Professor, Department of Physics, R.M.K.Engineering college, Kavaraipettai, Tamil Nadu, India
- Professor, Department of Computer Science and Engineering, Panimalar Engineering College, Chennai, Tamil Nadu, India
Abstract
The development of multifunctional polymer composite systems for intelligent thermal energy storage has gained significant attention due to the increasing demand for sustainable and autonomous thermal management technologies. In the present study, a wireless-integrated biopolymer–phase change material (PCM) composite module embedded with thermal feedback sensors was successfully fabricated and experimentally investigated for advanced thermal energy storage applications. Polylactic acid (PLA) was employed as the biodegradable polymer matrix, while paraffin wax served as the latent heat storage material. Graphite nanoplatelets were incorporated as conductive nanofillers to improve thermal conductivity and heat transfer characteristics within the composite structure. Embedded thermistor-based wireless sensing architecture enabled real-time thermal monitoring during charging and discharging operations. Differential scanning calorimetry analysis revealed stable melting and solidification transitions with excellent latent heat storage behaviour, while thermogravimetric analysis confirmed enhanced thermal stability of the polymer composite system. Thermal charging and discharging studies demonstrated efficient heat absorption, prolonged heat retention, and stable cyclic thermal performance. Scanning electron microscopy revealed homogeneous PCM dispersion, interconnected graphite nanoplatelet networks, and strong filler–matrix interfacial bonding within the composite structure. The synergistic integration of biodegradable polymer matrices, conductive reinforcements, latent heat storage materials, and embedded wireless sensing systems resulted in a multifunctional smart polymer composite suitable for autonomous thermal regulation applications. The developed composite module demonstrates strong potential for renewable energy storage, intelligent building materials, wearable thermal management systems, and next-generation IoT-enabled thermal energy platforms.
Keywords: polymer composite, nanoplatelet, thermal management, Differential scanning calorimetry, PCM dispersion
A Chandrashekhar, K. Arun, Om Prakash Sharma, Rathinamala S, Mallikarjunarao Dandu, M. Premalatha, P Joel Josephson, G.Nixon Samuel Vijayakumar, Rajendiran M. Smart Biopolymer–PCM Composite Modules with Embedded Wireless Thermal Sensing for Autonomous Energy Storage Applications. Journal of Polymer & Composites. 2026; 14(04):-.
A Chandrashekhar, K. Arun, Om Prakash Sharma, Rathinamala S, Mallikarjunarao Dandu, M. Premalatha, P Joel Josephson, G.Nixon Samuel Vijayakumar, Rajendiran M. Smart Biopolymer–PCM Composite Modules with Embedded Wireless Thermal Sensing for Autonomous Energy Storage Applications. Journal of Polymer & Composites. 2026; 14(04):-. Available from: https://journals.stmjournals.com/jopc/article=2026/view=246526
References
1. Zhou K, Ding R, Ma X, Lin Y. Printable and flexible integrated sensing systems for wireless healthcare. Nanoscale. 2024;16(15):7264-86.
2. Jia L, Li Y, Ren A, Xiang T, Zhou S. Degradable and recyclable hydrogels for sustainable bioelectronics. ACS Applied Materials & Interfaces. 2024 Jun 21;16(26):32887-905.
3. Appusamy S, Krishnan S, Gopikrishna M, Raman S. Bio-based materials for microwave devices: A review. Journal of Electronic Materials. 2021 Apr;50(4):1893-921.
4. Mirbakht SS, Golparvar A, Umar M, Kuzubasoglu BA, Irani FS, Yapici MK. Highly self-adhesive and biodegradable silk bioelectronics for all-in-one imperceptible long-term electrophysiological biosignals monitoring. Advanced Science. 2025 Feb;12(8):2405988.
5. Kalimuthu P, Gonzalez-Martinez JF, Ruzgas T, Sotres J. Highly stable passive wireless sensor for protease activity based on fatty acid-coupled gelatin composite films. Analytical Chemistry. 2020 Aug 31;92(19):13110-7.
6. Staples M, Daniel K, Cima MJ, Langer R. Application of micro-and nano-electromechanical devices to drug delivery. Pharmaceutical Research. 2006 May;23(5):847-63.
7. Staples M, Daniel K, Cima MJ, Langer R. Expert review. Pharmaceutical Research. 2006 May;23(5).
8. Shin JW, Kim DJ, Jang TM, Han WB, Lee JH, Ko GJ, Yang SM, Rajaram K, Han S, Kang H, Lim JH. Highly elastic, bioresorbable polymeric materials for stretchable, transient electronic systems. Nano-Micro Letters. 2024 Dec;16(1):102.
9. Janardhanan S, Delalic JZ, Catchmark J, Saini D. Development of biocompatible MEMS wireless capacitive pressure sensor. Journal of Microelectronics and Electronic Packaging. 2005 Oct 1;2(4):287-96.
10. Ngashangva L, Goswami P, Chakma B. Smart materials for developing sensor platforms. In: Advanced Materials and Techniques for Biosensors and Bioanalytical Applications. CRC Press; 2020. p. 47-68.
11. Shili M, Hammedi S, Chaoui H, Nouri K. A novel intelligent thermal feedback framework for electric motor protection in embedded robotic systems. Electronics. 2025 Sep 10;14(18):3598.
12. Tan YK. Energy harvesting autonomous sensor systems. CRC Press; 2013.
13. Musiał M, Lichołai L, Katunský D. Modern thermal energy storage systems dedicated to autonomous buildings. Energies. 2023 May 31;16(11):4442.
14. Fojtik M, Kim D, Chen G, Lin YS, Fick D, Park J, Seok M, Chen MT, Foo Z, Blaauw D, Sylvester D. A millimeter-scale energy-autonomous sensor system with stacked battery and solar cells. IEEE Journal of Solid-State Circuits. 2013 Jan 22;48(3):801-13.
15. Oudenhoven JF, Vullers RJ, van Schaijk R. A review of the present situation and future developments of micro-batteries for wireless autonomous sensor systems. International Journal of Energy Research. 2012 Oct 10;36(12):1139-50.
16. Ayrilmis N, Kanat G, Yildiz Avsar E, Palanisamy S, Ashori A. Utilizing waste manhole covers and fibreboard as reinforcing fillers for thermoplastic composites. J Reinf Plast Compos. 2025;44(17-18):1108-1118.
17. Almeshaal M, Palanisamy S, Murugesan TM, Palaniappan M, Santulli C. Physico-chemical characterization of Grewia monticola Sond fibers for prospective application in biocomposites. J Nat Fibers. 2022;19(17):15276-15290.
18. Palanisamy S, Mayandi K, Palaniappan M, Alavudeen A, Rajini N, Vannucchi de Camargo F, Santulli C. Mechanical properties of Phormium tenax reinforced natural rubber composites. Fibers. 2021;9(2):11.
19. Ramasubbu R, Kayambu A, Palanisamy S, Ayrilmis N. Mechanical properties of epoxy composites reinforced with Areca catechu fibers containing silicon carbide. BioResources. 2024;19(2).
20. Palanisamy S, Mayandi K, Dharmalingam S, Rajini N, Santulli C, Mohammad F, Al-Lohedan HA. Tensile properties and fracture morphology of Acacia caesia bark fibers treated with different alkali concentrations. J Nat Fibers. 2022;19(15):11258-11269.

Journal of Polymer & Composites
| Volume | 14 |
| 04 | |
| Received | 28/05/2026 |
| Accepted | 05/06/2026 |
| Published | 11/06/2026 |
| Publication Time | 14 Days |
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